Long-lived nonequilibrium states in quantum systems challenge the foundations of statistical mechanics. According to the ergodic hypothesis, isolated systems thermalize, but strong dissipation and interactions can give rise to stable nonequilibrium phases such as continuous time crystals (CTCs). These objects spontaneously break continuous time-translation symmetry, manifesting as undamped periodic oscillations. Experimentally, CTCs have been realized in ultracold atoms and spin systems, but their lifetimes were limited to milliseconds or minutes due to dephasing and heating.
The experiment used a cloud of cesium atoms in a vapor cell, excited by three lasers (852 nm, 1470 nm, 780 nm) to Rydberg states (49P3/2). An external radiofrequency field (8.2 MHz) modulated the Rydberg levels, creating Floquet dressed states and effective nonlinearity via long-range van der Waals interactions. The dissipative environment was controlled through spontaneous decay of Rydberg states and optical pumping. The optical response was recorded via probe beam transmission, allowing spectroscopic tracking of population dynamics. System parameters (RF field amplitude and laser detuning) were carefully tuned to drive the system into a regime with a nearly zero real part of the Liouvillian spectrum, minimizing decay.
At optimal parameters (field 45.6 V/m, detuning 0 MHz), self-oscillations at 15.03 kHz persisted for 16.95 hours (61,020 s), confirmed by continuous signal recording. The frequency spectrum remained stable with a maximum drift of just 30.5 Hz. Phase-wander analysis revealed superlinear growth of the mean square displacement (MSD ∝ $τ^1$.89), indicating correlated drift rather than simple diffusion. The Allan deviation reached a minimum of 5.3×10⁻⁵ at averaging times of 12,406 s, corresponding to an absolute frequency instability of about 0.79 Hz. The critical dependence of lifetime on field amplitude and laser detuning follows power laws, consistent with a theoretical model based on Liouvillian analysis.
Achieving a 16.95-hour CTC lifetime means the dissipative gap in the Liouvillian spectrum can be closed with high precision, realizing a practically dissipationless limit cycle. This proves the existence of stable nonequilibrium phases at macroscopic scales and enables precision sensing of weak fields through extremely long signal accumulation. The dissipationless nature implies nearly zero entropy production in the oscillatory regime. Moreover, the long-lived phase coherence could serve as a continuous quantum memory, storing information in the oscillation phase.
Further lifetime improvements may come from suppressing residual technical noise and cooling the atomic ensemble. Of particular interest is exploring the role of quantum fluctuations — transitioning from mean-field to a full quantum description, where finite entanglement may limit lifetime even with a closed Liouvillian gap. Coupling to mechanical oscillators or microwave resonators could also create hybrid time crystals.
The work impacts quantum metrology by providing a new type of oscillator with record stability, and quantum computing, where stable nonequilibrium states could serve as memory elements.
Immediate next steps include investigating the influence of finite temperature and interparticle correlations on phase diffusion, as well as experimentally demonstrating quantum enhancement in sensor applications.
The results directly touch on the arrow of time and thermalization, testing the applicability limits of the second law of thermodynamics in open quantum systems. Observing suppressed relaxation ties into the general principles of the fluctuation-dissipation theorem, making time crystals a testbed for nonequilibrium quantum statistics.
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What the work does
The study demonstrates a continuous time crystal in an ensemble of cesium Rydberg atoms with a record lifetime exceeding 16 hours. Self-sustained oscillations at 15.03 kHz were maintained through precise tuning of the dissipative environment and radio-frequency modulation, and phase diffusion analysis revealed superlinear growth of the mean squared displacement.
Where its strength is
The key achievement is the realization of a nearly dissipation-free limit cycle in a macroscopic system, confirmed by minimizing the real part of the Liouvillian spectrum and by record frequency stability. This paves the way for long-lived nonequilibrium phases as a resource for precision sensing.
Where it could go next
Worth trying
Nearby works in our archive
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Over 16.95 hours, the cesium atoms emitted and re-emitted about 9.2×$10^8$ oscillation cycles — if each cycle were a step, a pedometer would have counted the distance from Earth to the Moon and back.